Hot Chip, Made in the Dark
To some, this might blend in with a bunch of others of similar ilk, but what makes it stand out to me is the variety. They experiment, and have fun while doing so.
Autechre, Quaristice
First Autechre record I've liked in a long time, really dig this. In the experimental electronic genre.
The Last Shadow Puppets, The Age of the Understatement
I just really like the songwriting on this. A little bit old school (like older Scott Walker), but not as old school as She & Him.
A few more potentials:
Black Mountain, In the Future
5ive, Hesperus
Goldfrapp, Seventh Tree
Gutter Twins, Saturnalia
Kills, Midnight Boom
Magnetic Fields, Distortion
Mars Volta, The Bedlam in Goliath
She & Him, Volume One
Virgin Black, Requiem: Fortissimo